Robust evidence for reversal in the aerosol effective climate forcing trend

Quaas, J., Jia, H., Smith, C., Albright, A. L., Aas, W., Bellouin, N. ORCID: https://orcid.org/0000-0003-2109-9559, Boucher, O., Doutriaux-Boucher, M., Forster, P. M., Grosvenor, D., Jenkins, S., Klimont, Z., Loeb, N. G., Ma, X., Naik, V., Paulot, F., Stier, P., Wild, M., Myhre, G. and Schulz, M. (2022) Robust evidence for reversal in the aerosol effective climate forcing trend. Atmospheric Chemistry and Physics, 22 (18). pp. 12221-12239. ISSN 1680-7316 doi: 10.5194/acp-2022-295

Abstract/Summary

Anthropogenic aerosols exert a cooling influence that offsets part of the greenhouse gas warming. Due to their short tropospheric lifetime of only up to several days, the aerosol forcing responds quickly to emissions. Here we present and discuss the evolution of the aerosol forcing since 2000. There are multiple lines of evidence that allow us to robustly conclude that the anthropogenic aerosol effective radiative forcing – both aerosol-radiation and aerosol-cloud interactions – has become globally less negative, i.e. that the trend in aerosol effective radiative forcing changed sign from negative to positive. Bottom-up inventories show that anthropogenic primary aerosol and aerosol precursor emissions declined in most regions of the world; observations related to aerosol burden show declining trends, in particular of the fine-mode particles that make up most of the anthropogenic aerosols; satellite retrievals of cloud droplet numbers show trends in regions with aerosol declines that are consistent with these in sign, as do observations of top-of-atmosphere radiation. Climate model results, including a revised set that is constrained by observations of the ocean heat content evolution show a consistent sign and magnitude for a positive forcing relative to 2000 due to reduced aerosol effects. This reduction leads to an acceleration of the forcing of climate change, i.e. an increase in forcing by 0.1 to 0.3 W m−2, up to 12% of the total climate forcing in 2019 compared to 1750 according to IPCC.

Item Type	Article
URI	https://reading-clone.eprints-hosting.org/id/eprint/107151
Identification Number/DOI	10.5194/acp-2022-295
Refereed	Yes
Divisions	Science > School of Mathematical, Physical and Computational Sciences > Department of Meteorology
Publisher	Copernicus Publications
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